Palladium-Catalyzed Regioselective Synthesis of 3-Arylindoles from N-Ts-Anilines and Styrenes

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초록

A Pd-catalyzed intermolecular oxidative annulation between N-Ts-anilines and styrenes was developed. This method offers a straightforward and robust approach to a wide range of 3-arylindoles using readily available starting materials with good functional-group tolerance and high regioselectivity and efficiency. Further elaboration of the products obtained from this process provided access to highly functionalized and structurally diverse indoles, for example, 3-(indol-3-yl)carbazoles, 1,9-dihydropyrrolo-[2,3-b]carbazoles, and 3'-aryl-3,5'-biindoles.

키워드

C-H activationhomogeneous catalysisindolespalladiumregioselectivityC-H ACTIVATIONAEROBIC OXIDATIVE AMINATIONUNUSUAL 1,2-ARYL MIGRATION3-SUBSTITUTED INDOLESDIRECT ACCESSANNULATION2-ALKENYLANILINESALKENESALKYNESFUNCTIONALIZATIONS
제목
Palladium-Catalyzed Regioselective Synthesis of 3-Arylindoles from N-Ts-Anilines and Styrenes
저자
Youn, So WonKo, Tae YunJang, Young Ho
DOI
10.1002/anie.201702205
발행일
2017-06
유형
Article
저널명
Angewandte Chemie - International Edition
56
23
페이지
6636 ~ 6640