Pt-Catalyzed Hydrative Cyclization of 2-Enynylbenzaldehydes and Its Application to Faveline Synthesis

  • Oh, Chang Ho
  • Lee, Sung Min
  • Hong, Chang Seop
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초록

Various 2-[6-en-1-ynyl]benzaldehydes and their analogues were successfully cyclized via Huisgen-type [3+2] cycloaddition to the tetracyclic platinum-carbene complex, which would subsequently undergo hydration to afford the tricyclic products in good yields with excellent stereoselectivities. This hydrative cyclization was also applied to the faveline synthesis.

키워드

CONTAINING CARBONYL YLIDES5+2 CYCLOADDITIONO-ALKYNYLBENZALDEHYDESGENERATIONINSERTIONTANDEM(+/-)-DEOXOFAVELINEVINYLCYCLOPROPANESBENZOCYCLOHEPTENESBENZANNULATION
제목
Pt-Catalyzed Hydrative Cyclization of 2-Enynylbenzaldehydes and Its Application to Faveline Synthesis
저자
Oh, Chang HoLee, Sung MinHong, Chang Seop
DOI
10.1021/ol100255z
발행일
2010-03
유형
Article
저널명
Organic Letters
12
6
페이지
1308 ~ 1311