Improved electrochemical performances of LiM0.05Co0.95O1.95F0.05 (M = Mg, Al, Zr) at high voltage

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초록

Metal and F co-substituted LiM0.05Co0.95O1.95F0.05 (M = Mg, Al, Zr) cathode materials were successfully synthesized via a solid-state reaction. XRD measurements showed that cobalt and oxygen sites in LiCoO2 are successfully substituted for metal (Mg, Al, Zr) and fluorine, respectively. The co-substituted materials exhibited stable cycling performance, improved rate capability, and thermal stability compared to pristine LiCoO2. Furthermore, Co dissolution tests revealed that fluorine substitution stabilizes the cathode surface and thus suppresses Co dissolution. Among the materials, LiM0.05Co0.95O1.95F0.05 showed the best electrochemical and thermal properties.

키워드

Cathode materialLithium batteriesMetal and fluorine substitutionHigh voltageCOATED LINI0.5MN1.5O4 SPINELLITHIUM SECONDARY BATTERIESCATHODE MATERIALSCYCLING BEHAVIOR4.5 VFLUORINE SUBSTITUTIONINTERCALATION CATHODEION BATTERIESLICOO2CELLS
제목
Improved electrochemical performances of LiM0.05Co0.95O1.95F0.05 (M = Mg, Al, Zr) at high voltage
저자
Jung, Hun-GiGopal, Nulu VenuPrakash, JaiKIM, DONG WONSun, Yang Kook
DOI
10.1016/j.electacta.2012.02.057
발행일
2012-04
유형
Article
저널명
Electrochimica Acta
68
페이지
153 ~ 157