Separation of Co(II) Over Ni(II) from Chloride Leached Solution of Spent Li-Ion Batteries Using Cyphos IL104

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초록

The hydrometallurgical separation of cobalt and nickel was achieved from HCl leached solution of spent Li-ion batteries, while applying Cyphos IL104 as a potential extractant. Cobalt extraction significantly increases with increasing Cyphos IL104 and Cl− ion concentrations, and equilibrium pH (pHeq). Under the optimized condition of 0.8 mol·L−1 Cyphos IL104, 3.0 mol·L−1 Cl− ions, pHeq value 5.0, and O/A ratio of 2/3 could extract >99% Co with only 3% Ni into the organic phase. The back-extraction of cobalt performed with 2.0 mol·L−1 H2SO4 solution yielded 99.95% stripping efficiency and was crystallized to obtain high-pure CoSO4.xH2O crystals.

키워드

Hydrometallurgical recyclingIonic liquidLi-ion batteriesChlorine compoundsCobalt compoundsExtractionHydrometallurgyIonsLeachingLithium compoundsLithium-ion batteriesNickel compoundsRecyclingBack extractionCl- ionsCobalt and nickelsCobalt extractionExtractantsHydrometallurgical recyclingIon concentrationsIon equilibriumOptimized conditionsOrganic phaseIonic liquids
제목
Separation of Co(II) Over Ni(II) from Chloride Leached Solution of Spent Li-Ion Batteries Using Cyphos IL104
저자
Ilyas, SadiaKim, HyunjungSrivastava, Rajiv Ranjan
DOI
10.1007/978-3-031-22765-3_11
발행일
2023-02
유형
Conference paper
저널명
Minerals, Metals and Materials Series
페이지
107 ~ 116