1-Aminoanthraquinone as an electro-polymerizable additive to improve the cycling performance of a Na₃V₂(PO₄)₂F₃cathode

  • Park, Myung-Soo
  • Choi, Jin-Yi
  • Veerasubramani, Ganesh Kumar
  • Kim, Dong-Won
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초록

A small amount of 1-aminoanthraquinone (AAQ) was used as an electro-polymerizable additive in a liquid electrolyte. AAQ was electrochemically oxidized to form a thin conductive poly(1-aminoanthraquinone) (PAAQ) layer on a sodium-ion cathode material, Na3V2(PO4)(2)F-3 (NVPF), at approximately 4.0 V during the initial charging processes. The resulting PAAQ layer provided an effective conduction pathway in the NVPF electrode, and thus enhanced the cycling performance in terms of the discharge capacity, cycling stability and rate capability. Our study demonstrates a simple and efficient approach to boost the electrochemical performance of a NVPF cathode for sodium-ion batteries.

키워드

Electrolyte additiveConductive polymerElectro-oxidative polymerizationSodium-ion batteryPoly(1-aminoanthraquinone)AdditivesCathodesElectric dischargesElectrolytesMetal ionsSodium-ion batteries1-AminoanthraquinoneCharging processCycling performanceCycling stabilityDischarge capacitiesElectrochemical performanceLiquid electrolytesRate capabilities
제목
1-Aminoanthraquinone as an electro-polymerizable additive to improve the cycling performance of a Na₃V₂(PO₄)₂F₃cathode
저자
Park, Myung-SooChoi, Jin-YiVeerasubramani, Ganesh KumarKim, Dong-Won
DOI
10.1016/j.elecom.2020.106829
발행일
2020-10
유형
Article
저널명
Electrochemistry Communications
119
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1 ~ 6

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