Synthesis and characterization of Pt-, Pd-, and Ru-promoted Ni-Ce0.6Zr0.4O2 catalysts for efficient biodiesel production by deoxygenation of oleic acid

  • Jeon, Kyung-Won
  • Shim, Jae-Oh
  • Cho, Jae-Wan
  • Jang, Won-Jun
  • Na, Hyun-Suk
  • ... Jeon, Byong Hun
  • 외 4명
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초록

Herein, we prepared Pt-, Pd-, and Ru-promoted Ni-Ce0.6Zr0.4O2 catalysts with improved oleic acid deoxygenation performance and investigated their physicochemical properties by N-2 adsorption-desorption, X-ray diffraction (XRD), NH3 temperature-programmed desorption (NH3-TPD), and X-ray photoelectron spectroscopy (XPS). Among the above catalysts, the highest oleic acid conversion, C-9-C-17 selectivity, and oxygen removal efficiency were observed for Pt/Ni-Ce0.6Zr0.4O2, which was mainly ascribed to its highest surface defect oxygen fraction and acidity.

키워드

Ni-Ce0.6Zr0.4O2Noble metalPromoterDeoxygenationOleic acidHIGH-QUALITY DIESELSTEARIC-ACIDFATTY-ACIDSJET-FUELOILDECARBOXYLATIONHYDROTREATMENTPATHWAYSBIOMASSNI
제목
Synthesis and characterization of Pt-, Pd-, and Ru-promoted Ni-Ce0.6Zr0.4O2 catalysts for efficient biodiesel production by deoxygenation of oleic acid
저자
Jeon, Kyung-WonShim, Jae-OhCho, Jae-WanJang, Won-JunNa, Hyun-SukKim, Hak-MinLee, Yeol-LimJeon, Byong HunBae, Jong WookRoh, Hyun-Seog
DOI
10.1016/j.fuel.2018.09.078
발행일
2019-01
유형
Article
저널명
Fuel
236
페이지
928 ~ 933