N-Arylation of Sterically Hindered NH-Nucleophiles: Copper-Mediated Syntheses of Diverse N-Arylindole-2-carboxylates

Citations

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초록

Indole-carboxylates are N-arylated with 2-bromopyridines using stoichiometric copper(II) oxide/potassium carbonate to give various N-(2-pyridyl)-substituted indole-2-carboxylates and with bromobenzenes using stoichiometric copper(I) iodide/N,N'-dimethylethylenediamine to give various N-(substituted phenyl)-substituted indole-2-carboxylates. These results expand the scope of metal-catalyzed N-arylation using heterocyclic amines with steric bulk and weak nucleophilicity.

키워드

copperN-arylationindolescopper-mediated synthesisheterocyclic aminesmetal-catalyzedCROSS-COUPLING REACTIONSNITROGEN-CONTAINING HETEROCYCLESC-NFISCHER INDOLIZATIONARYL HALIDESINDOLESPALLADIUMEFFICIENTULLMANNDERIVATIVES
제목
N-Arylation of Sterically Hindered NH-Nucleophiles: Copper-Mediated Syntheses of Diverse N-Arylindole-2-carboxylates
저자
Lee, JinyongChoi, Ji HyeShin, SeunghoonHeo, Jung-NyoungLim, Hwan Jung
DOI
10.1055/s-0035-1560065
발행일
2015-11
유형
Article
저널명
Synthesis
47
21
페이지
3301 ~ 3308